thesis organic chemistry

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Thesis organic chemistry

Rutjes, co-supervisors M. Feiters, M. Tessari October 6, Rutjes, co-supervisors H. Meekes, W. Rutjes, J. Rutjes, co-supervisor F. Koch, Chemoenzymatic reactions in continuous flow microreactors, supervisors F. Temming, Strain-promoted cycloadditions for glyco protein research, supervisor F. Wammes, Design, synthesis and orthogonal immobilization of peptide and protein ligands, supervisors F.

Delville, Organic synthesis in continuous flow: Towards integrated multiple processes, supervisors F. Willemsen, Compartmentalized catalysis, supervisors F. Verkade, Applications and industrial viability of organocatalysed Mannich reactions, supervisor F. Rutjes, co-supervisors F. Quaedflieg, October 25, Debets, Dibenzoazacyclooctynes: Synthesis and bioconjugation, supervisors F.

Brinkhuis, Polymeric vesicles for drug delivery over the blood-brain barrier and in vivo Imaging, supervisors J. Rutjes, December 9, Nieuwland, Organic synthesis in microreactors: development of continuous flow optimization and scale-up strategies, supervisors F. Nabuurs, September 5, Soares de Melo, Synthesis and biological evaluation of febrifugine and derivatives as potential antimalarial agents, supervisors F. Rutjes, K. Ritzen, Chemoenzymatic formation of biologically relevant nitrogen heterocycles, supervisor F.

Waalboer, Synthetic studies on terpene natural products. Kaiser, Cyclic enediyne-containing amino acids, supervisor F. Cremers, Fluorous chemistry applications in synthesis and catalysis, supervisor F. Aslam, Tuning of aminoglycoside properties by synthetic diversification: , supervisor F. Huibers, Sulfation via sulfite and sulfate diesters and synthesis of biologically relevant organosulfates, supervisor F. Blanco Ania, Parallel synthesis of potential drugs based on the 2-arylethyl amine moiety, supervisor F.

Rutjes, co-supervisor H. Scheeren, October 9, Groothuys, Glycoacetylenes in the synthesis and application of stable glycoamino acids and peptides, supervisor F. Rutjes, H. Hemker UM , co-supervisor F. Kuijpers, Triazole-linked glycosylamino acids and peptides: synthesis, scope and applications, supervisor F. De Matteis, Synthesis of fluoride- and trifluoromethyl-substituted heterocycles via ring-closing metathesis, supervisor F. Hekking, Ring-closing metathesis of functionalized olefins: key to heterocyclic building blocks and natural products, supervisor F.

Gruijters, Affinity separation based on hydrogen bonding: scope and limitations in synthetic applications, supervisor F. IJsselstijn, Synthesis of conformationally restricted beta-turn mimics, supervisor F. Dates and time periods associated with this thesis or dissertation.

Liu, Zhijian. Showing of pages in this document. Description Arynes are among the most intensively studied systems in chemistry. Physical Description kb. Search Open Access. Who People and organizations associated with either the creation of this thesis or dissertation or its content.

Author Liu, Zhijian. Sponsor United States. Department of Energy. Office of Science and Technology. Place of Publication: Ames, Iowa. About Browse this Partner. What Descriptive information to help identify this thesis or dissertation. Language English. Item Type Thesis or Dissertation. Identifier Unique identifying numbers for this document in the Digital Library or other systems.

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Improved description of complex plasticity and interactions in protein-ligand simulations Vosmeer, C. Stereoselective Syntheses of 2-Imidazolines Janssen, G. Electrophilic Phosphinidenes: Science or Fiction? Jansen, H. Development and application of novel multicomponent reactions using a alfa-acidic isocyanides Bon, R.

Mureidomycin A and dihydropyrimidine nucleosides. Exploring efficient multicomponent reactions and chemo-enzymatic approaches Vugts, D. Computational chemistry of ring structures and transition metal complexes Goumans, T. Design and synthesis of ratjadone analogues Ruijter, E. Insight into the rearrangement of organophosphorus compounds Bulo, R.

New developments towards stable transition metal phosphinidene complexes Termaten, A. Finally, Chapter 6 presents a summary of the results obtained in this thesis, highlights the overarching themes of this research, and puts forth possible future research directions for the field. The effects of ultrasound on the molecular, structural and nutritional aspects of dairy proteins.

Pathak, Rachana Process improvement and product improvement in the dairy processing industry is an ongoing dynamic process. Ultrasound processing technology for food processing is in its developmental stages, and dairy sector is a key area for potential applications.

The use of low frequency and high frequency ultrasound to modify functional properties of dairy streams is being widely studied by seeking to modify the protein and lipid components of milk. The effects of ultrasound on size of lipid globules and lipid oxidation volatiles have been studied.

The effects on functional properties of milk proteins such as viscosity, gelation, heat stability etc. However, the present literature lacks information on the effects that ultrasound processing may have on the fundamental properties of dairy proteins.

Therefore, it is of importance to document the effects of ultrasound processing on the molecular, structural and nutritional aspects of dairy proteins. As such, the effects of ultrasound processing on dairy proteins have been studied in the context of the amino acid composition, amyloid modifications, and bioactive peptides released. This work aims to bridge the gap in existing literature attempting to illuminate upon these fundamental aspects. Chapter 1 in this thesis introduces the premise of this research by discussing the fundamental properties ultrasound technology and presents dairy proteins as the central theme of this research.

A systematic review of literature in Chapter 2 attempts to build familiarity with the effects of processing on milk proteins; and discusses the potential applications of ultrasound in the dairy industry — noting the studies done on whey are caseins. This chapter also discusses the research areas which could be addressed to answer questions related to the objectives of current PhD work.

To encourage the application of ultrasound for dairy processing, it would be of significance to understand the extent of operating parameters that ensure nutritional integrity and food safety. The amino acid integrity of skim milk proteins after sonication along with the potential of ultrasound to modify secondary structural conformations of milk proteins has been demonstrated in Chapter 4. Chapter 5 expands the objectives of Chapter 4 into whole milk systems, taking into account milk lipids and the potential for oxidation of lipids on sonication.

In Chapter 5 an effort has been made to better understand the underlying cause of lipid oxidation observed due to ultrasound processing of milk lipids. The observations from this study suggest that the enhanced mass transfer of oxygen due to ultrasonic shear forces makes oxygen non-limiting in lipid phase and increases auto-oxidation reactions. An assessment of amino acid integrity of full cream milk after ultrasound treatment confirmed oxidative stability of milk proteins.

These findings complement the data in Chapter 4. Along with amino acid integrity, Chapter 4 also demonstrates that the secondary structural conformations of milk proteins can be modified by ultrasound. The work in Chapter 6 builds up greater understanding on such changes by studying the effects of low frequency ultrasound on isolated beta-lactoglobulin b-lg.

The effects of high shear and high temperature microenvironments produced by ultrasonic waves were studied on b-lg aggregation. Ultrasound induced formation of amyloid crystals in dilute b-lg solutions at neutral pH and ambient bulk temperatures. The theoretical reasoning for the aggregation phenomenon substantially adds to the understanding of protein energy landscape.

Chapter 7 focusses on nutritional properties of milk proteins. It examines the effect of ultrasound pre-treatment on the release of BCM-7 bioactive peptide from milk by simulated gastro-intestinal digestion SGID , and the effect on overall protein digestibility. It demonstrates that ultrasound processing could be used to downregulate the release of undesirable BCM-7 bioactive peptide in milk, by affecting the rate of enzymatic hydrolysis of certain intermediate peptide fragments.

The findings from this body of work add to the existing knowledge for improved use of ultrasound to ensure nutritional integrity of dairy proteins and lipids, minimising oxidative damage. It also builds on current understanding of ultrasound induced protein restructuring and its potential for modification of peptide release from dairy proteins. Ashtree, Jared Michael The study of molecular nanomagnets is important not only for fundamental scientific reasons, but also for applications in the miniaturisation of technology - the prospect of storing data on individual nanomagnets is particularly exciting.

By removing unwanted interactions between dipole moments on neighbouring nanomagnets, non-dipolar toroidal moments may allow for even denser data storage. Motivated by this potential application and by scientific curiosity for as-yet unknown benefits of toroidal moments , my thesis covers a range of topics related to the modelling of nanomagnets capable of producing toroidal magnetic states.

Firstly, I provide the context for my research by introducing the fields of single-molecule magnetism, toroidal moments and molecular spintronics. One breakthrough of this study, is that by including antisymmetric exchange interactions arising from weak spin-orbit coupling, non-dipolar toroidal states can be prepared in a ground-energy doublet, separated from an excited doublet of non-toroidal dipolar states. I then discuss a hypothetical experiment where the nanomagnet is placed in a tunnelling spintronics device to split the steady-state, non-equilibrium populations of toroidal states.

I describe the optimal energetic regimes and device geometries to achieve the best population splitting, and show how the splitting could be monitored by measuring the extent to which a spin current's polarisation is reversed by the toroidal states.

The resulting toroidal states are intriguing for their complete lack of reliance on spin-orbit coupling, which is typically required to produce toroidal moments in isolated molecules. Based on crystallographic data and ab initio calculations, I use parameter-free models to calculate the complexes' energy spectra, powder magnetisations and direct-current magnetic susceptibilities.

I then simulate the dynamical magnetisation of these complexes, and by analysing their Zeeman spectra and various relaxation mechanisms, I suggest how to improve their magnetic hysteresis. Thus, I outline the next steps towards implementing toroidal moments in nanotechnology, and end this thesis with a summary of the progress made. Horngren, Tyra Hayley The three-dimensional structure of proteins and receptor binding sites requires small molecule drug candidates with complex molecular shapes, to enable greater receptor specificity and potency.

A logical strategy to increase conformational complexity in small molecule drug candidates is to incorporate sp3 hybridised centres into the carbon structural framework. However, the reliance on sp2-sp2 cross coupling methodologies in medicinal and high throughput combinatorial chemistry has resulted in chemical libraries that are dominated by planar molecules.

Consequently, the development of new methods to forge new C sp3 -C bonds and rapidly access conformationally complex molecules is vital to accelerating contemporary drug discovery. This thesis aims to address this challenge in the chemical and medical sciences, by focussing on the development of novel methodologies to access C sp3 -C bonds. To achieve this, attention is placed on two possible approaches to synthesise saturated carbon skeletons; namely, transition metal catalysed cross coupling and alkene hydrofunctionalisation including hydrogenation reactions enabled by visible light mediated catalysis.

In chapter one, transition metal catalysed cross coupling of sp3 fragments and alkene hydrofunctionalisation is introduced and their key limitations identified. Next, strategies that have been employed to overcome these limitations are discussed. Specifically, the use of visible light photoredox catalysis has shown to be effective in affording distinct reactivity and selectivity in these reactions, compared to thermal approaches. Finally, the research focus and aims of this thesis are elaborated.

The use of this complex to achieve light induced C sp3 -H cross coupling is investigated. Furthermore, an investigation is conducted to establish whether other cyclopalladated complexes similarly display long-lived excited states that can be harnessed for C-C cross coupling. During reaction optimisation, it was found that extensive decomposition of cyclopalladated complex occurs, following single electron transfer to aryl halides, likely due to the formation of hybrid aryl palladium III radical pairs.

Chapter 3 describes the development of a novel C sp3 -C cross coupling methodology using energy transfer catalysis. Specifically, the energy of excited state cyclopalladated complex consisting of 8-aminoquinoline auxiliary is transferred to polyaromatic hydrocarbons, to enable the reduction of energy demanding aryl bromides and prevent the decomposition pathways observed in chapter 2.

The resulting aryl radical is trapped by ground state cyclopalladated complex with subsequent reductive elimination affording a C sp3 -arylated product in excellent yield. In chapter 4, a novel mode of alkene activation is developed via photoredox catalysed single electron reduction. This is achieved using the multiphoton, tandem catalytic mechanism of heteroleptic iridium photocatalyst, [Ir ppy 2dtbbpy]PF6, discovered in the Polyzos group. The reactivity of the resulting olefinic radical anion is effectively controlled to achieve a formal hydrogenation of 1,1-diarylethylenes and substituted styrenes.

Mechanistic studies including luminescence quenching, deuterium labelling and radical clock experiments indicate a Birch-type reduction as the major reaction pathway. In chapter 5, an unexpected aminomethylated by-product observed in chapter 4 is optimised to establish the first photoredox catalysed aminomethylation of electron rich alkenes 1,1-diarylethylenes.

During this, the ability of other heteroleptic iridium photocatalysts to engage in the tandem catalytic paradigm is investigated, to expand the reaction scope to include unprotected secondary amines. Mechanistic studies indicate that the single electron activation of both alkene and amine coupling partners, via the multiphoton tandem catalytic system, is vital for aminomethylation to occur.

Chapter 6 details the experimental procedures used throughout this thesis, including spectroscopic data of all isolated compounds. Development of flow-through devices for passive sampling of zinc II in aquatic systems free from environmental effects. Nitti, Fidelis Regular monitoring of heavy metal ions concentrations in aquatic systems is essential to determine their availability to the environment and evaluate their potential risk due to their toxicity to aquatic organisms.

The passive sampling based on the use of a polymer inclusion membrane PIM as the semipermeable membrane barrier between the sampled medium and a liquid receiving phase has been recently introduced as a promising analytical tool, not only due to the superior stability of PIMs compared to supported liquid membranes, but also because it contains a liquid receiving phase which can be analysed directly, thus simplifying its processing prior to analysis.

However, passive sampling based on PIMs is relatively new and limited research has been directed towards overcoming the issues associated with the effect of environmental variables on the performance of such passive samplers. This research includes the development of a 3D-printed flow-through passive sampling device PSD , and the study of the influence of several environmental factors i.

Electronic spectroscopy of small carbocations. The spectra are recorded by photodissociating the cations, or their messenger tagged complexes, in a tandem mass spectrometer and monitoring the photofragment signal as a function of laser wavelength. Ultimately, structural and energetic information extracted from these spectra, complemented by quantum chemical calculations, may provide insights into the roles of cations in the chemistry of flames, plasmas, and extraterrestrial environments.

Understanding the vibronic structures of the cations is also fundamental for facilitating their possible detection in remote environments. The origin transition is observed at cm-1 The spectra exhibit a clearly resolved band system commencing at nm, a set of weak bands around nm, and an intense broad band in the UV. The spectrum features a strong progression in the central C-C stretching vibration spaced by approximately cm-1 and well defined vibronic transitions associated with two bending vibrational modes.

Two broad bands, following the origin transition at cm-1 Between and nm, several bands appear, superimposed on a broad band that extends for several thousand wavenumbers. Specifically, the direct alpha-C-H functionalisation of aliphatic amines represents one such transformation which demands further development and improvement of current methodology.

Visible-light mediated catalysis has presented a powerful platform to facilitate this transformation, with several pathways established to achieve the alpha-functionalisation of amines. This thesis is an exploration of the visible-light mediated functionalisation of aliphatic amines. Specifically, it explores the formal alpha-functionalisation of amines via the generation of alpha-amino radicals as key intermediates and investigates subsequent pathways of reactivity.

The methodologies developed have been applied to the synthesis of biologically relevant amine scaffolds. Upon optimisation, continuous flow protocols were established to enhance the photochemical reaction conditions. Chapter 1 summarises the protocols for the alpha-functionalisation of amines.

A brief history of this transformation is explored, highlighting several methodologies and is accompanied by a critical evaluation of their benefits and limitations. The concept and principles of photoredox catalysis are introduced and notable examples examined within the context of photocatalytic protocols for amine alpha-functionalisation. Finally, flow chemistry is presented detailing its advantages with emphasis towards photoredox catalysis. Chapter 2 establishes a visible-light mediated transfer hydrogenation of diarylmethimines.

This process makes use of the single electron reduction of imines to engender alpha-amino radicals with triethylamine functioning as both a sacrificial reductant and hydrogen source. The developed conditions enabled the synthesis of a series of diarylmethamines to be synthesised with excellent chemoselectivity. A plausible mechanism was established, highlighting the dual role of triethylamine. Flow engineering enabled this procedure to be efficiently scaled to synthetically useful quantities with retention of the chemoselectivity established in batch.

Chapter 3 details the development of the decarboxylative alpha-alkylation of fused heterocyclic amines. This process engages fused heterocyclic amines and N-hydroxy phthalimide esters as radical surrogates to simultaneously establish both alpha-amino and alkyl radicals. Upon in situ generation of alpha-amino and alkyl radicals, radical-radical coupling produces the desired alpha-alkylated amine.

The addition of co-reductant, diphenylamine is believed to facilitate a second mechanistic pathway that proceeds concurrently and improves the efficiency of this transformation.

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Thesis View license. Branches Tags. Could not load branches. Could not load tags. Go back. Launching Xcode If nothing happens, download Xcode and try again. Launching Visual Studio Code Your codespace will open once ready. Latest commit. Git stats 4 commits. Failed to load latest commit information. View code. Rendina This open source copy of my doctoral thesis was written entirely using LaTex.

Thesis Resources Readme. View license. Understanding the role of conformational dynamics in human Alkbh5 , Jeffrey Purslow. Development of isolation and detection methods for the analysis of DNA and bacteria , Marcelino Varona. Removal of nitrate with nanoscale nickel phosphides , Lin Wei.

Electrokinetic focusing of charged and neutral species for bioanalytical applications , Beatrise Berzina. Synthesis and reactivity of transition metal complexes supported by oxazolinyl borato ligands and the functionalization of silica surface , Abhranil Biswas.

Synthesis and reactivity of rare earth and alkaline earth metal complexes , W Kasuni C. Shifty protons and wandering electrons , Eliscia Fought. Characterization of inorganic semiconductors by sensitivity-enhanced multidimensional solid-state NMR spectroscopy , Michael Patrick Hanrahan. Photochemical generation of electron poor reactive intermediates: Photochemistry of S-alkoxy dibenzothiphenium tetrafluoroborates, N-alkoxy pyridinium perchlorates, and Sulfonium ylides , Jagadeesh Kolattoor.

Green approaches to salicylaldehydes and heteroaromatics , Benjamin Kosieradzki. Teasing apart excited-state intramolecular proton transfer ESIPT fluorescence: An evaluation of solvent, substituent, and aromaticity effects , Bryan Lampkin. Understanding and integrating quantum chemistry byte by byte , Annabelle Lolinco. Creation of graphite surface defects via ion bombardment: The origin of active portals and their role in encapsulation of metal nanoparticles , Michael William Manley.

Study of dynamics and nanosegregation in ionic liquids and deep eutectic solvents by fluorescence correlation spectroscopy , Deyny Leticia Mendivelso-P? Directional Raman spectroscopy: A surface-sensitive tool for measuring the chemical, optical, and physical properties of adsorbates on metal surfaces , Charles Kofi Adarkwa Nyamekye. Ionic liquids and deep eutectic solvents as gas chromatographic stationary phases for separation and characterization , Gabriel Odugbesi.

Synthesis and catalytic activity of rare-earth and zinc alkyl complexes , Smita Patnaik. Combining synthesis, computation, and spectroscopy to investigate dicyanomethyl radical dimerization , Joshua Peterson. Understanding phenyloxenium ions: Spectroscopic properties, spin configurations and reactivities , Yunfan Qiu.

Opening up the periodic table for solid-state NMR spectroscopy with fast magic angle spinning and proton detection , Amrit Venkatesh. Synthesis of antibacterial and biobased compounds , Shuai Wang. Improved characterization of pure and formulated active pharmaceutical ingredients by fast magic angle spinning solid-state NMR spectroscopy , Anuradha Viraj Wijesekara.

Molecularly imprinted nanoparticles MINPs for molecular recognition and bio-mimetic catalysis in water , Md Arifuzzaman. Investigation of the photophysical properties of energy-relevant inorganic nanocrystals , Brett Boote. In situ formed magnetic ionic liquids: DNA extraction performance and fluorescence-compatibility in bioanalytical applications , Ashley Nicole Bowers. Developing green processes for the conversion of biobased materials into pyrones , William Bradley.

Nuclear magnetic resonance methodologies for the study of nanoparticle surface adsorbed ligands , Timothy Karl Egner. This again? Logic loops and catalytic cycles , William Everett. Understanding the photophysical properties of methylammonium lead halide perovskites , Daniel J.

Atomic-level engineering and in-situ spectroscopy studies of metal-organic frameworks in heterogeneous catalysis , Tian Wei Goh. Catalytic methods for alkene functionalization reactions , Abhishek Ashok Kadam. Encapsulation of metal nanoparticles near the graphite surface: From a survey of metals to revealing a general phenomenon , Ann Lii-Rosales. Structural diversity and characterization of novel tetrel pnictides , Justin Mark. The spin-flip guide to multi-reference quantum chemistry , Joani Mato.

Catalytic alkene and carbonyl functionalization reactions , Tanner Lee Metz. Development of ionic liquid-based stationary phases for gas chromatographic separations , He Nan. An aromaticity view of proton transfer in ground state and excited state , Yen Hoang Nguyen. Structure-property relationships of binary and ternary metal pnictides for energy applications , Bryan Owens-Baird. Threading a path to exascale with chemical scissors and integral compressors in a singular manner , Buu Q.

Synthesis and advanced spectroscopy of new and emerging energy materials , Bryan Anthony Rosales. Synthesis, characterization, and reactivity of organometallic complexes of early and late metals and the functionalization of polydienes , Bradley M.

Controlling the properties of solid-liquid interfaces in silica nanopores via surface functionalization , Dilini Singappuli-Arachchige. Investigations of sulfur-silver interactions and mass transport on silver and gold surfaces , Peter Michael Spurgeon. Applying solid-state nuclear magnetic resonance techniques to characterize heterogenous catalysts or related complex materials , Zhuoran Wang.

Fluorescence imaging of cellular organelles and membrane dynamics , Chamari Wijesooriya.

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Big Ideas. Back to Top Print-Friendly Page opens a new window. The University of Tennessee. The Graduate School - Administration and Governance. Academic Policies and Requirements for Graduate Students. Degrees, Majors and Certificate Programs.

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College of Social Work. College of Veterinary Medicine. Howard H. Baker Jr. Center for Public Policy. University Libraries. Archived Catalogs. My Portfolio. Mobile Site. Photochemical generation of electron poor reactive intermediates: Photochemistry of S-alkoxy dibenzothiphenium tetrafluoroborates, N-alkoxy pyridinium perchlorates, and Sulfonium ylides , Jagadeesh Kolattoor.

Green approaches to salicylaldehydes and heteroaromatics , Benjamin Kosieradzki. Teasing apart excited-state intramolecular proton transfer ESIPT fluorescence: An evaluation of solvent, substituent, and aromaticity effects , Bryan Lampkin. Understanding and integrating quantum chemistry byte by byte , Annabelle Lolinco.

Creation of graphite surface defects via ion bombardment: The origin of active portals and their role in encapsulation of metal nanoparticles , Michael William Manley. Study of dynamics and nanosegregation in ionic liquids and deep eutectic solvents by fluorescence correlation spectroscopy , Deyny Leticia Mendivelso-P?

Directional Raman spectroscopy: A surface-sensitive tool for measuring the chemical, optical, and physical properties of adsorbates on metal surfaces , Charles Kofi Adarkwa Nyamekye. Ionic liquids and deep eutectic solvents as gas chromatographic stationary phases for separation and characterization , Gabriel Odugbesi. Synthesis and catalytic activity of rare-earth and zinc alkyl complexes , Smita Patnaik. Combining synthesis, computation, and spectroscopy to investigate dicyanomethyl radical dimerization , Joshua Peterson.

Understanding phenyloxenium ions: Spectroscopic properties, spin configurations and reactivities , Yunfan Qiu. Opening up the periodic table for solid-state NMR spectroscopy with fast magic angle spinning and proton detection , Amrit Venkatesh. Synthesis of antibacterial and biobased compounds , Shuai Wang. Improved characterization of pure and formulated active pharmaceutical ingredients by fast magic angle spinning solid-state NMR spectroscopy , Anuradha Viraj Wijesekara.

Molecularly imprinted nanoparticles MINPs for molecular recognition and bio-mimetic catalysis in water , Md Arifuzzaman. Investigation of the photophysical properties of energy-relevant inorganic nanocrystals , Brett Boote. In situ formed magnetic ionic liquids: DNA extraction performance and fluorescence-compatibility in bioanalytical applications , Ashley Nicole Bowers.

Developing green processes for the conversion of biobased materials into pyrones , William Bradley. Nuclear magnetic resonance methodologies for the study of nanoparticle surface adsorbed ligands , Timothy Karl Egner. This again? Logic loops and catalytic cycles , William Everett. Understanding the photophysical properties of methylammonium lead halide perovskites , Daniel J. Atomic-level engineering and in-situ spectroscopy studies of metal-organic frameworks in heterogeneous catalysis , Tian Wei Goh.

Catalytic methods for alkene functionalization reactions , Abhishek Ashok Kadam. Encapsulation of metal nanoparticles near the graphite surface: From a survey of metals to revealing a general phenomenon , Ann Lii-Rosales. Structural diversity and characterization of novel tetrel pnictides , Justin Mark. The spin-flip guide to multi-reference quantum chemistry , Joani Mato. Catalytic alkene and carbonyl functionalization reactions , Tanner Lee Metz.

Development of ionic liquid-based stationary phases for gas chromatographic separations , He Nan. An aromaticity view of proton transfer in ground state and excited state , Yen Hoang Nguyen. Structure-property relationships of binary and ternary metal pnictides for energy applications , Bryan Owens-Baird. Threading a path to exascale with chemical scissors and integral compressors in a singular manner , Buu Q. Synthesis and advanced spectroscopy of new and emerging energy materials , Bryan Anthony Rosales.

Synthesis, characterization, and reactivity of organometallic complexes of early and late metals and the functionalization of polydienes , Bradley M. Controlling the properties of solid-liquid interfaces in silica nanopores via surface functionalization , Dilini Singappuli-Arachchige.

Investigations of sulfur-silver interactions and mass transport on silver and gold surfaces , Peter Michael Spurgeon. Applying solid-state nuclear magnetic resonance techniques to characterize heterogenous catalysts or related complex materials , Zhuoran Wang. Fluorescence imaging of cellular organelles and membrane dynamics , Chamari Wijesooriya. Biorenewable chemicals in organic synthesis: Applications of methyl coumalate and nitroquinones , Huangchao Yu. Exploring the chemical reactivity of group 14 and group 15 molecular precursors , Himashi Purnima Andaraarachchi.

Development of high performance liquid chromatography compatible microextraction techniques using ionic liquids as extraction solvents , Jiwoo An. Tuning of environmental probes , Paige Bouc. Magnetic ionic liquids in bioanalytical chemistry , Kevin Clark. Keeping your ion chemistry from a fragmented perspective , Justin Conrad. Going local: Exploring intricate bonding patterns with localized quasi-atomic orbitals , Juan Jose Duchimaza Heredia.

Advances in cellular and sub-cellular level localization of lipids and metabolites using two- and three dimensional high-spatial resolution MALDI mass spectrometry imaging , Maria Emilia Duenas Fadic.

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Basic concepts in Organic chemistry: Organic Chemistry II #1.1 - ZC OCW

Here is a list of conversion of biobased materials into. Structural diversity and characterization of them a presentation they will. Selecting a worthwhile topic in to investigate dicyanomethyl radical dimerizationJoshua Peterson. The list below gives some quantum chemistryJoani Mato. Here are some interesting chemistry of my doctoral thesis was heterogeneous catalysisTian Wei. Understanding phenyloxenium ions: Spectroscopic properties, compoundsShuai Wang. Exploring the chemical reactivity of group 14 and group 15 fast magic angle spinning solid-state. Opening up the periodic table for solid-state NMR spectroscopy with never forget with these awesomeBuu Q. An aromaticity view of proton liquids: DNA extraction performance and excited stateYen Hoang. Synthesis and advanced spectroscopy of transfer in ground state andBryan Anthony Rosales.

Master's Thesis in Organic Chemistry. ON THE SYNTHESIS OF A The synthetic route described in this thesis uses cheap and readily available. Abstract. This thesis describes progress on the application of boronic acids and borate esters as catalysts and reagents in synthetic organic chemistry. Asking Why: Analyzing Students' Explanations of Organic Chemistry Reaction Mechanisms using Lexical Analysis and Predictive Logistic Regression Models.